Footballer Harrison Solomon, 22, decided to leave the show after being involved in one of the most dramatic love triangles in the show's history.
The Derby lad, who is based in Miami, has been flip-flopping between Toni Laites and Lauren Wood for days - leaving both of them in tears along the way.
Harrison left the villa late on Thursday night and will be heading home soon.
A source said: "It's been a momentous few days for Harrison and ultimately he has decided to quit.
"Everyone was so shocked and people were crying and hugging him.
"He worked through everything with the ITV duty of care team and is making his way home to his family now."
Last night's episode included a tense challenge which saw the couples decide who should place first, second and third after a number of questions were put to the public.
Among them were "which couple is coasting?", "who is the biggest game player?" and "who is in the most one-sided relationship?".
There was a familiar theme with Harrison and Toni, Dejon Williams and Meg Moore, and Harry Cooksley and Helena Ford making up the top three in most categories.
The day before, Harrison got emotional after seeing the devastation he was causing.
Controversially, he made a plea to Toni ahead of the latest recoupling to pick him, despite having had sex with Lauren the night before.
‘Grow up!’ rage Love Island fans as controversial boy reveals he doesn’t know how to complete basic life task
Toni's decision to choose him blindsided their exes Cach Mercer and Lauren, with both left sobbing after being embarrassed in front of their friends.
Earlier that day, she'd told Lauren she was done with Harrison.
Sitting by the fire pit, she said: “He's all yours, girlfriend.
"I'm removing myself from this.
WHO are the latest bombshells heading into the spin-off villa?
The Sun exclusively reported the identities of the six beauties heading into the ITV2 spin-off villa, after it was teased during last week's episode.
The Love Island newbies were seen strolling into the compound clad in swimwear - with one already having a connection to Harry.
On the show's official Instagram page it teased: "Amor the merrier… who’s ready for Casa Amor?" and now we can report the full line-up.
“This is getting f**king ridiculous and it's making me nasty.
“He's lying to both of us. I can't keep doing this.”
Though he was warned by multiple people that he now needed to focus on Toni, Harrison couldn't help himself.
He complimented Lauren's looks last night when he saw her wearing a red bikini and refused to close the door completely.
She was even caught helping him floss his teeth, which proved to be the final straw for Toni, who accused him of constantly making her look stupid.
4
4
Footballer Harrison Solomon, 22, decided to leave the show after being involved in one of the most dramatic love triangles in the show's history. Harrison has sensationally quit the Love Island villa Harrison and Toni reached the end of the road last nightCredit: Eroteme The Derby lad, ...
Recently, the new relationship hit the rocks when Andy was twice quizzed by police over bust-ups with Lou ANDY Carroll and Lou Teasdale look loved up in their new pics amid "fears they won't last" and a Greek holiday bust up. Andy was ...
The newsreader was in her usual slot as the programme's anchor on Thursday's edition of the ITV lunchtime chat show when she and her co-stars discussed the news that 16 and 17-year-olds will now be able to vote. When Kelly's turn came to speak, ...
Like a phoenix rising from the ashes (in head-to-toe designer, body tea, mind you), Porsha Williams has returned to The Real Housewives of Atlanta to bring the looks, the drama, and, of course, the party. Porsha falls into the precious category of Housewives (alongside Phaedra, Dorinda, ...
EX-Love Island star Nathalia Campos has certainly been living a life of luxury since her time in the villa – now boasting a brand new £97k Porsche. The stunning star shared pics and video of the big reveal of the fancy ...